To sort references alphabetically in your bibliography (i.e. sorted by first author's last name), from the Export dropdown, select Export Options and choose Citation Style :
apacite (bibtex) if you would like a natural APA-looking citation of the form "Rodriguez (2011)"
alpha (bibtex) if you'd like a citation of the form "[Rod11]"
plain (bibtex) if you would like a numbered citation of the form "[1]"
All the above Citation Styles produce a reference list sorted alphabetically.
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